Terahertz metasurfaces have great applications for efficient terahertz modulation, but there are still problems in designing terahertz metadevices in terms of complexity and inefficiency. Herein, we demonstrate an inversely-designed terahertz metasurface with double electromagnetically induced transparency (EIT)-like windows by incorporating a particle swarm optimization (PSO) algorithm with the finite-difference time-domain method. We prepared and tested the metadevices, and the experimental terahertz signals are close to the designed results. By hybridizing amorphous germanium film with the inversely-designed metasurface, two EIT-like windows, including transmission and slow-light effect, exhibit ultrafast modulation behavior in 25 ps excited by a femtosecond laser. The modulation depths of transmission in two transparency windows are 74% and 65%, respectively. The numerical simulations also illustrate the ultrafast dynamic process and modulation mechanism, which match well with the experiment results. Our work thus offers opportunities for designing other objective functions of the terahertz metadevice.

Metasurface plays a key role in various terahertz metadevices, while the designed terahertz metasurface still lacks flexibility and variety. On the other hand, inverse design has drawn plenty of attention due to its flexibility and robustness in the application of photonics. This provides an excellent opportunity for metasurface design as well as the development of multifunctional, high-performance terahertz devices. In this work, we demonstrate that, for the first time, a terahertz metasurface supported by the electromagnetically induced transparency (EIT) effect can be constructed by inverse design, which combines the particle swarm optimization algorithm with the finite-difference time-domain method. Incorporating germanium (Ge) film with inverse-designed metasurface, an ultrafast EIT modulation on the picosecond scale has been experimentally verified. The experimental results suggest a feasibility to build the terahertz EIT effect in the metasurface through an optimization algorithm of inverse design. Furthermore, this method can be further utilized to design multifunctional and high-performance terahertz devices, which is hard to accomplish in a traditional metamaterial structure. In a word, our method not only provides a novel way to design an ultrafast all-optical terahertz modulator based on artificial metamaterials but also shows the potential applications of inverse design on the terahertz devices.

Helicity-dependent ultrafast spin current generated by circularly polarized photons in topological materials holds the crux to many technological improvements, such as quantum communications, on-chip communication processing and storage. Here, we present the manipulation of helicity-dependent terahertz emission generated in a nodal line semimetal candidate Mg₃Bi₂ by using photon polarization states. The terahertz emission is mainly ascribed to the helicity-dependent photocurrent that is originated from circular photogalvanic effects, and the helicity-independent photocurrent that is attributed to linear photogalvanic effect. Our work will inspire more explorations into novel nodal line semimetals and open up new opportunities for developing ultrafast optoelectronics in the topological system.

We experimentally demonstrate for the first time an active all-optical ultrafast modulation of electromagnetically induced transparency-like effect in a hybrid device of sapphire/Si/metamaterial. From numerical simulations, it can be deducted that the tuning process is attributed to the coupling between the dark mode existing in split-ring resonators and the bright mode existing in cut wire resonators. The transmission amplitude modulation is accompanied by the slow-light effect. In addition, the ultrafast formation process is measured to be as fast as 2 ps. This work should make an important contribution to novel chip-scale photonic devices and terahertz communications.

Metamaterials play an important role in the modulation of amplitude and group delay in the terahertz (THz) regime on account of their optical properties, which are rare in natural materials. Here an ultrafast anisotropic switch of the plasmon-induced transparency (PIT) effect is experimentally and numerically demonstrated by metamaterial devices composed of two pairs of planar split-ring resonators and a pair of closed-ring resonators. By integration with a germanium (Ge) film, a recovery time of 3 ps and a decay constant of 785 fs are realized in the metadevice. Stimulated by the exterior optical pump, the PIT windows at different frequencies are switched off with an excellent property of slow light for vertical and horizontal THz polarizations, realizing an astonishing modulation depth as high as 99.06%. This work provides a new platform for ultrafast anisotropic metadevices tunable for amplitude and group delay.

Active control of metamaterial properties with high tunability of both resonant intensity and frequency is essential for advanced terahertz (THz) applications, ranging from spectroscopy and sensing to communications. Among varied metamaterials, plasmon-induced transparency (PIT) has enabled active control with giant sensitivity by embedding semiconducting materials. However, there is still a stringent challenge to achieve dynamic responses in both intensity and frequency modulation. Here, an anisotropic THz active metamaterial device with an ultrasensitive modulation feature is proposed and experimentally studied. A radiative-radiative-coupled PIT system is established, with a frequency shift of 0.26 THz in its sharp transparent windows by polarization rotation. Enabled by high charge-carrier mobility and longer diffusion lengths, we utilize a straightforwardly spin-coated MAPbI3 film acting as a photoactive medium to endow the device with high sensitivity and ultrafast speed. When the device is pumped by an ultralow laser fluence, the PIT transmission windows at 0.86 and 1.12 THz demonstrate a significant reduction for two polarizations, respectively, with a full recovery time of 561 ps. In addition, we numerically prove the validity that the investigated resonator structure is sensitive to the optically induced conductivity. The hybrid system not only achieves resonant intensity and frequency modulations simultaneously, but also preserves the all-optical-induced switching merits with high sensitivity and speed, which enriches multifunctional subwavelength metamaterial devices at THz frequencies.